Diesel Emission Inventory

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Abstract: Atmospheric pollution is created by emissions from a variety of sources. Emission inventories are performed to identify the significance of particular sources to the overall pollution situation. Diesel engines are significant contributors to the overall NOx and PM pollution.

Diesel Engines and Air Pollution

Today’s emissions from mobile sources, including cars, trucks, and off-road vehicles, are estimated to be responsible for about 50% of nationwide NOx emissions, about 40-50% of HC (or VOC) emissions, and as much as 80-90% of CO emissions in urban areas. Similar contributions are seen in the USA and in other developed countries, including Europe and Japan. A large portion of these emissions comes from gasoline fueled cars and light trucks. However, the relative importance of NOx and PM emissions from diesel engines has been increasing. This increase has been caused by (1) the introduction of three-way catalyst technology for spark ignited engines in the 1980s, which lowered gasoline NOx emissions, and (2) increasing trends in diesel vehicle population and diesel fuel usage.

There is an increased penetration of diesel fueled vehicles in the passenger car market in Europe. With the exception of Sweden, where diesels almost disappeared, sales of diesel cars in most countries show an increasing trend. As illustrated in Table 1 [295][909], the proportion of diesel cars sold in 2002 in Austria, Belgium and France exceeded 60% of all new automobiles in these countries.

**Table 1**
Market Penetration of New Diesel Cars in Europe, % of New Cars Sold
	1980	1985	1990	1995	2002*
Austria	3.3	13.7	25.7	42.6	69.0
Belgium	13.8	26.4	32.9	46.8	63.5
France	9.9	15.0	33.0	46.5	62.0
Germany	8.0	22.1	10.8	14.6	37.0
Italy	8.1	25.1	7.3	10.3	42.0
Sweden	6.0	2.2	0.6	2.8	6.7
UK	0.4	3.6	6.4	20.2	22.5
Europe (weighted average)	7.2	15.6	13.9	22.1	39.3
* new car registrations January-June 2002

Even though diesel passenger cars are not used in the USA (market penetration 0.03% in 1994), the consumption of diesel fuel relative to the total fuel consumption by all highway vehicles has been steadily increasing. The same increasing trend has been noted in Japan (Figure 1 [295]).

Figure 1. Diesel Fuel Consumption As a Fraction of Total Highway Fuel Consumption

In the past, when diesel fuels contained high levels of sulfur, diesel engines were also important contributors to the sulfur dioxide (SO₂) emission inventory. Lowering the fuel sulfur level from about 0.3-0.5% to 0.05%, which occurred in the mid-1990s in the USA and in Europe, was an effective means of controlling SO₂ emissions from diesel fueled engines. In 1999, the contribution of highway diesel engines to the nationwide SO₂ inventory in the USA is only 0.6%. However, the contribution of non-road engines, which still used high sulfur diesel fuel, amounted to 2.7% [541]. The relative importance of diesels in SO₂ pollution may be higher in countries which still use diesel fuels of high sulfur content.